• 综合性科技类中文核心期刊
    • 中国科技论文统计源期刊
    • 中国科学引文数据库来源期刊
    • 中国学术期刊文摘数据库(核心版)来源期刊
    • 中国学术期刊综合评价数据库来源期刊
JI Shu-lan, YANG Yuan-yuan, QIN Zhen-ping, LI Jian-ting, SUN Tong. Isothermal Adsorption of Steroid Estrogens onto Aerobic Granular Sludge[J]. Journal of Beijing University of Technology, 2009, 35(11): 1537-1542. DOI: 10.3969/j.issn.0254-0037.2009.11.017
Citation: JI Shu-lan, YANG Yuan-yuan, QIN Zhen-ping, LI Jian-ting, SUN Tong. Isothermal Adsorption of Steroid Estrogens onto Aerobic Granular Sludge[J]. Journal of Beijing University of Technology, 2009, 35(11): 1537-1542. DOI: 10.3969/j.issn.0254-0037.2009.11.017

Isothermal Adsorption of Steroid Estrogens onto Aerobic Granular Sludge

More Information
  • Received Date: June 09, 2008
  • Available Online: December 09, 2022
  • In order to research the adsorption of estrone (E1) , 17β-estradiol (E2) and 17α-ethynylestradiol (EE2) onto aerobic granular sludge, the adsorption balance time and the biosorption behavior under different temperatures were studied.The experiment data were fit with Freundlich equation and Langmuir equation.The structure of AGS was observed by SEM.The results show that the adsorption equilibrium is within 40 min, and the maximum adsorption capacity (qmax) decreases with increasing temperature.The qmax s of E1、E2、EE2 are 60.98, 58.82, and 82.64 μg/g respectively at 20 ℃.This adsorption process is in conformity with the isothermal adsorption equation of Langmuir and Freundlich with R2 correlation coefficient between 0.93~0.98 and 0.92~0.98, respectively.The results of SEM show that there are changes in the internal and external morphology of AGS.
  • [1]
    TERNES T A, STUMPF M, MUELLER J, et al.Behavior and occurrence of estrogens in municipal sewage treatmentplants-I[J].Sci Total Environ, 1999, 225 (1-2) :81-90.
    [2]
    METCALFE C D, METCALFE T L, KIPARISSIS Y, et al.Estrogenic potency of chemicals detected in sewage treatmentplant effluents as determined by in vivo assays with Japanese medaka (Oryzias latipes) [J].Environ Toxicol Chem, 2001, 20 (2) :297-308.
    [3]
    BARONTI C, CURINI R, D’ASCENZO G, et al.Monitoring natural and synthetic estrogens at activated treatment plantsand in receiving river water[J].Environ Sci Technol, 2000, 34 (24) :5059-5066.
    [4]
    TABATA A, KASHIWA S, OHNISHI Y, et al.Estrogenic influence of estradiol-17h, p-nonylphenol and bisphenol A onJapanese Medaka (Oryzias iatipes) at detected environmental concentrations[J].Water Sci Technol, 2001, 43 (2) :109-116.
    [5]
    JOHNSON A C, BELFOID A, DI C A.Estimating steroid estrogens inputs into activated sludge treatment works andobservations on their removal from the effluent[J].Sci Total Environ, 2000, 256 (2-3) :163-173.
    [6]
    邓南圣, 吴峰.环境中的内分泌干扰物[M].北京:化学工业出版社, 2004.
    [7]
    MILES-RICHARDSON S R, KRAMER V J, FITZGERALD S D, et al.Effects of Waterborne exposure of 17β-estradiol onsecondary sex characteristics and gonads of fathead minnows (Pimephales promelas) [J].Aquatic Toxicology, 1999, 47 (2) :129-145.
    [8]
    LIU Yu, YANG Shu-fang, XU Hui, et al.Biosorption kinetics of cadmium (Ⅱ) on aerobic granular sludge[J].ProcessBiochemistry, 2003, 38 (7) :997-1001.
    [9]
    杨学耀, 李进, 李久义, 等.好氧颗粒污泥吸附重金属Cd (Ⅱ) 的研究[J].工业用水与废水, 2007, 38 (1) :28-31.YANG Xue-yao, LI Jin, LI Jiu-yi, et al.Adsorption of heavy metal Cd (Ⅱ) by aerobic granular sludge[J].Industrial Water&Wastewater, 2007, 38 (1) :28-31. (in Chinese)
    [10]
    姚磊, 叶正芳, 王中友, 等.好氧颗粒污泥对Pb2+的吸附特性研究[J].科学通报, 2007, 52 (20) :2434-2438.YAO Lei, YE Zheng-fang, WANG Zhong-you, et al.Study on biosorption of Pb2+on aerobic granular sludge[J].ChineseScience Bulletin, 2007, 52 (20) :2434-2438. (in Chinese)
    [11]
    曾庆玲, 李咏梅, 顾国维.厌氧与缺氧污泥对17β-雌二醇吸附性能的研究[J].环境科学, 2007, 28 (9) :1981-1986.ZENG Qing-ling, LI Yong-mei, GU Guo-wei.Adsorption Characteristics of 17β-estradiol to Anaerobic and Anoxic Sludge[J], Environmental Science, 2007, 28 (9) :1981-1986. (in Chinese)
    [12]
    任海燕.甾体雌激素的检测及降解菌的选育和生物强化应用[D].北京:北京工业大学环境与能源工程学院, 2006.REN Hai-yan.Analysis of steroid estrogens and isolation of degradation strain and bioaugmentation application[D].Beijing:College of Environment and Energy Engineering of Beijing University of Technology, 2006. (in Chinese)
    [13]
    LAI K M, JOHNSON K L, SCRIMSHAW M D, et al.Binding of waterborne steroid estrogens to solid phases in river andestuarine systems[J].Environ Sci Technol, 2000, 34 (18) :3890-3894.

Catalog

    Article views (11) PDF downloads (3) Cited by()

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return